Quantum coherence, which quantifies the superposition properties of a quantum state, plays an indispensable role in quantum resource theory. A recent theoretical work [Phys. Rev. Lett. 116, 070402 (2016) [CrossRef] ] studied the manipulation of quantum coherence in bipartite or multipartite systems under the protocol local incoherent operation and classical communication (LQICC). Here we present what we believe is the first experimental realization of obtaining maximal coherence in the assisted distillation protocol based on a linear optical system. The results of our work show that the optimal distillable coherence rate can be reached even in one-copy scenario when the overall bipartite qubit state is pure. Moreover, the experiments for mixed states showed that distillable coherence can be increased with less demand than entanglement distillation. Our work might be helpful in remote quantum information processing and quantum control.